Optimization of high-order harmonic generation by genetic algorithm and wavelet time-frequency analysis of quantum dipole emission
نویسندگان
چکیده
We present an ab initio three-dimensional quantum study of the coherent control of high-order harmonic generation ~HHG! processes in intense pulsed laser fields by means of the genetic algorithm optimization of the laser-pulse amplitude and phase. Accurate time-dependent wavefunction and HHG power spectrum are obtained by the time-dependent generalized pseudospectral method and wavelet transform is used to obtain the dynamical phase associated with the dipole-emission time profile. It is shown that ‘‘intra-atomic’’ dynamical phase matching on the sub-optical cycle, attosecond, time scale can be achieved, leading to nearly perfect constructive interference between different returning electronic wave packets and marked improvement in both emission intensity and purity of a given harmonic order.
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